new porous crystals of extended metal catecholates

结构信息. V. The pellets of Ni3(2,3,6,7,10,11-hexaiminotriphenylene)2, which has recently been developed, show n-type thermoelectric transport, dependent on . His present research interests mainly focus on the design and synthesis of electrically conductive metal-organic frameworks (MOF) membranes for energy conversion devices. Extended; New Porous Crystals; Similar works. Read more about CAT-1; CAT-5. All Since 2017; Citations: 31016: 16033: h-index: 78: 57: i10-index: 231: 190: 0. New Porous Crystals of Extended Metal-Catecholates Chemistry . Sheberla D, . Just create or connect your ORCID iD. Chem. During which, (TPHS) 6− was formed. Where size matters Mohamad Hmadeh, Zheng Lu, Zheng Liu, Felipe Gándara, Hiroyasu Furukawa, Shun Wan, Veronica Agustyn, Rui Chang, Lei . Metal-organic framework (MOF-5), a prototype of a new class of porous materials and one that is constructed from octahedral Zn-O-C clusters and benzene links, was used to demonstrate that its three-dimensional porous system can be functionalized with the organic groups -Br, -NH 2, -OC 3 H 7, -OC 5 H 11, -C 2 H 4, and -C 4 H 4 and that its pore . 2018 , 140, 4812-4819 DOI: 10.1021/jacs.7b08174 New porous crystals of extended metal-catecholates. 24, 3511-3513. . You You Wang, Qing Jin, Shi Xin Liu, Chao Guo, Yuan Yuan Liu, Bin Ding, Xiang Xia Wu, Yan Li, Zhao Zhou Zhu, A series of two-dimensional microporous triazole-functionalized metal-organic frameworks with the new multi-dentate ligand 1-(4-aminobenzyl)-1,2,4-triazole: single-crystal-to-single-crystal transformation, structural diversity and . 1) Boden, N.; Borner, R. C.; Bushby, R. J.; Cammidge, A. N.; Jesudason, M. V. Liquid Crystals 1993, 15(6), 851-858 Conductive metal-organic framework (MOF) materials have been recently considered as effective electrocatalysts. Mater. New Porous Crystals of Extended Metal-Catecholates. Most of the excess value is distributed in the range from 0.5 to 1.5 mol g −1 and the excess amounts for 252 structures are higher than those of Co-CMP (1.802 mol g −1 ), which can capture and. 分子量. 6 7408 through metal-catecholate linkages.19 In contrast to the archetypical carboxylate-based MOFs, metal-catecholates dis-play electron transport due to favorable orbital overlap between the metal ion (e.g., Fe, V) and the catechol.20−22 Here, a new 3D anionic metal-catecholate framework [Fe 6 (OH 2) 4 (CoPc) 3] 6−, termed MOF-1992, is constructed A new family of porous crystals was prepared by combining 1H-1,2,3-triazole and divalent metal ions (Mg, Mn, Fe, Co, Cu, and Zn) to give six isostructural metal-triazolates (termed MET-1 to 6). @article{osti_1052884, title = {New Porous Crystals of Extended Metal-Catecholates}, author = {Hmadeh, Mohamad and Lu, Zheng and Liu, Zheng and Gándara, Felipe and Furukawa, Hiroyasu and Wan, Shun and Augustyn, Veronica and Chang, Rui and Liao, Lei and Zhou, Fei and Perre, Emilie and Ozolins, Vidvuds and Suenaga, Kazu and Duan, Xiangfeng and Dunn, Bruce and Yamamto, Yasuaki and Terasaki . Sign in. Get my own profile. This approach is elaborated to make metal-catecholates (CATs) and metal triazolates (METs). Am. Wang M et al. 10.1021/cm301194a . Sign in. New Porous Crystals of Extended Metal-Catecholates. * "New Materials are Powering the Battery Revolution." The Conversation, 4 October 2018. Titanium coordination compounds: from discrete metal complexes to metal-organic frameworks. The relatively high conductivity shown by these materials demonstrates that targeting low-dimensional pathways is not mandatory for achieving efficient charge transport. . Chem. If you notice any inaccuracies, please sign in and mark papers as correct or incorrect matches. Chemistry of Materials,2012,24(18):3511 − 3513. doi: 10.1021/cm301194a [32] CAMPBELL M G, LIU S F, SWAGER T M, et al. Claim your Citation Index profile in order to display more information about you and gain access to Libraries services. <italic>Chem Mater</italic>, 2012, 24(18): 3511 doi: 10.1021/cm301194a [27] Sheberla D, Sun L, Blood-Forsythe M A, et al. 324.28. . The thin film not only can be precisely prepared in nanometer scale (20-70 nm), but also shows the pin-hole-free smooth surface. Am. Chem. University of New South Wales, School of Chemical Engineering, Sydney, Australia. Chemistry of Materials 24 (18), 3511-3513 , 2012 Chem. New porous crystals of extended metal catecholates Hmadeh, Mohamad Lu, Zheng Liu, Zheng Gandara, Felipe Show others and affiliations 2012 (English) In: Chemistry of Materials, ISSN 0897-4756, E-ISSN 1520-5002, Vol. 22 high-probability publications. Metal-organic frameworks (MOFs) are a promising class of porous hybrid organic/inorganic materials with a wide variety of applications in energy storage and conversion, 1-3 1. 性质说明. Herein we report on the thermoelectric properties of a two-dimensional coordination polymer pellets. Done. 2. If you identify any major omissions or other inaccuracies in the publication list, please let us know. Manthiram. Mater. The Cu-MOF demonstrates superior electrocatalytic activity for glucose oxidation under alkaline pH conditions. * "New Porous Crystals of Extended Metal-Catecholates." Chemistry of . Mohamad Hmadeh, Zheng Lu, . The incorporation of Ti(IV) units made MOF-901 useful in the photocatalyzed polymerization of methyl methacrylate (MMA). Crossref Google Scholar. Fe, V) and the catechol.20,21,22 Here, a new 3D anionic metal- Metal ions and organic linker self-assemble to form a framework which can be 1D/2D/3D in connectivity. metal-catecholate frameworks, a class of MOFs that are constructed through metal-catecholate linkages.19 In contrast to the archetypical carboxylate-based MOFs, metal-catecholates display electron transport due to favorable orbital overlap between the metal ion (e.g. Hmadeh M et al 2012 New porous crystals of extended metal-catecholates Chem. According to this, covalent long chain molecules ("Makromoleküle") do exist and are composed of a sequence of linearly connected repeat units . Mater. My profile My library Metrics Alerts. Three-Dimensional Metal-Catecholate Frameworks and Their Ultrahigh Proton Conductivity . New porous crystals of extended metal-catecholates. J. Mohamad Hmadeh, Zheng Lu, . 1) 4877-80-9 溶于DMF、DMSO等. Am. You are looking at the Reticular Chemistry Naming and Numbering Database created to be useful in identifying, naming, and numbering new crystalline, extended frameworks. Chem. A new family of porous crystals was prepared by combining 1H-1,2,3-triazole and divalent metal ions (Mg, Mn, Fe, Co, Cu, and Zn) to give six isostructural metal-triazolates (termed MET-1 to 6). Two-dimensional (2D) metal-organic frameworks (MOFs) 1-5 are novel 2D materials formed by metal atoms and polar organic molecules, and have aroused wide interest among researchers 6-16 due to their advantages of low cost, chemical tenability, easy fabrication, and mechanical flexibility. Settings. In the past decade, advances in electrically conductive metal-organic frameworks (MOFs) and MOF-based electronic devices have created new opportunities for the development of next-generation sensors. As an excellent non-enzymatic . Matheu R et al. As shown in figure . "On-surface Synthesis of Highly Oriented Thin Metal-organic Framework Films through Vapor-assisted Conversion." J. The amorphous porous salt exhibited greater porosity than its building blocks, due to the removal of non-porous counter-ions from the original structure, displaying a S BET of 496 m 2 g -1 for the amorphous porous salt, against the S BET of 416 m 2 g -1 and non-porous of the individual Me 2-ZrMOP and SO 3-CuMOP, respectively (Figure 7b). Authors. Chem. 10.1021/cm301194a . Three-dimensional phthalocyanine metal-catecholates for high electrochemical carbon dioxide reduction. New Porous Crystals of Extended Metal-Catecholates Abstract To date, the links of robust and highly porous metal organic frameworks (MOFs) have been largely limited to carboxylate, (1) imidazolate, (2) other azolates, (3) or sulfonate. The physical properties of several types of metal-organic frameworks (MOFs), which comprise an organic linker and metal ions/clusters, have been studied using tunable and well-defined porous specimens to explore their applicability in gas adsorption and separation ().Currently, their electrical properties (2-4), such as their conductivity (5-10), magnetism (11, 12), photonic . Chemistry of Materials, 24(18), 3511-3513. doi:10.1021/cm301194a . A Metal-Organic Framework Based on a Nickel Bis(dithiolene) Connector: Synthesis, Crystal Structure, and Application as an Electrochemical Glucose Sensor. These new crystalline materials, termed metal-catecholates (M-CATs), were characterized by X-ray diffraction techniques (single crystal for Co-CAT-1, and powder for Ni-CAT-1) and high- resolution transmission electron microscopy (HR-TEM) studies (for Ni-CAT-1). In this paper, a dual-ligand design strategy is demonstrated to modulate the performance of the electronically conductive metalorganic frameworks (EC-MOFs) thin film with a spray layer-by-layer assembly method. New porous crystals of extended metal-catecholates[J] . Pseudocapacitors Based on Hierarchically Porous Nanowire Composites." ACS Nano, 6 (2012) . which assemble into 2D porous extended frameworks, which may exhibit similar nontrivial properties. Mater. Metal-catecholates (Ni/Co-CATs, M = Co, Ni, Cu, etc.) Email address for updates. A Metal-Organic Framework Based on a Nickel Bis(dithiolene) Connector: Synthesis, Crystal Structure, and Application as an Electrochemical Glucose Sensor. New Porous Crystals of Extended Metal-Catecholates | Chemistry of Materials RETURN TO ISSUE Communication NEXT New Porous Crystals of Extended Metal-Catecholates Mohamad Hmadeh †‡ , Zheng Lu †‡ , Zheng Liu § , Felipe Gándara †‡ , Hiroyasu Furukawa †‡ , Shun Wan †‡ , Veronica Augustyn ⊥ , Rui Chang ⊥ , Lei Liao ‡ , Fei Zhou ⊥ , Emilie Perre ⊥ , A two-dimensional polymer (2DP) is a sheet-like monomolecular macromolecule consisting of laterally connected repeat units with end groups along all edges. New Porous Crystals of Extended Metal-Catecholates. 1. 分子式. High electrical conductivity in Ni-3(2, 3, 6, 7, 10, 11-hexaiminotriphenyl-ene)(2), a semiconducting metal-organic graphene analogue. School of Information and Control Engineering, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China Conductive MOFs are a class of metal−organic frameworks with intrinsic ability of electronic conduction. 2019. Commun. Soc., 2015, 137, 15394-15397 DOI: 10.1021/jacs.5b10999 Abstract: A series of three-dimensional (3D) extended metal catecholates (M-CATs) was synthesized by combining . Paper: Three-Dimensional Metal-Catecholate Frameworks and Their Ultrahigh Proton Conductivity Authors: N. T. T. Nguyen, H. Furukawa, F. Gándara, C. A. Trickett, H. M. Jeong, K. E. Cordova, and O. M. Yaghi Citation: J. New porous crystals of extended metal-catecholates. 24, 3511-3513 (2012 . New Porous Crystals of Extended Metal-Catecholates. Thermodynamics and kinetics of O2 adsorption and its impacts on structural features and conductive behavior of 2D π-stacked layered metal-organic frameworks (MOFs) are studied using periodic PBE-D3. New porous crystals of extended metal-catecholates M Hmadeh, Z Lu, Z Liu, F Gándara, H Furukawa, S Wan, V Augustyn, . * "New Materials are Powering the Battery Revolution." The Conversation, 4 October 2018. Am. Hala Assi† a, Georges Mouchaham† a, Nathalie Steunou a, Thomas Devic * ab and Christian Serre * ac a Institut Lavoisier, UMR CNRS 8180, Université de Versailles St-Quentin en Yvelines, Université Paris Saclay, 45 Avenue des Etats-Unis, 78035 Versailles Cedex, France b Institut des Matériaux . 近几十年来，金属有机框架（MOF）发展迅速，热度有增无减，是材料领域无愧的当红辣子鸡。但是导电MOF打破了MOF材料几乎不导电的桎梏，完美地结合了有机材料的结构可控和无机材料的长程有序，再加上特有的高电子迁移率，导电MOF可谓集万千宠爱于一身。2009年第一例导电MOF报道以来，这类材料 . FigShare Provided original full text link. Molecular electrocatalysts can mediate fast, selective CO 2 reduction in a flow cell. 141:17081-17085. Metal-organic frameworks (MOFs) / porous coordination polymers (PCPs) have emerged as a new family of conductive solid materials with outstanding performances in a wide variety of applications, including fuel cells, batteries, supercapacitors, catalysts, sensors, electronics, thermoelectrics, and spintronics. T. Qiu, Z. Liang, W. Guo, H. Tabassum, S. Gao, and R. Zou, " Metal-organic framework-based materials for energy conversion and storage," ACS Energy Lett. Chem. Chem. Augustyn. New Porous Crystals of Extended Metal-Catecholates M. Hmadeh, Z. Lu, Z. Liu, F. Gándara, H. Furukawa, S. Wan, V. Augustyn, R. Cheng, L. Liao, F. Zhou, E. Perre, V . 2019. Metal-organic frameworks (MOFs) are a class of materials constructed by the combination of organic linkers and metal ions to produce extended networks that possess pores and cavities of adjustable size and shape (Furukawa et al., 2013).MOFs are among the most porous materials known, some of them possessing BET and Langmuir specific surface area values higher than 6000 m 2 g . For 2D or quasi-2D crystals with three-fold symmetry, generally, . Full text. Chemiresistive sensor arrays from conductive 2D metal-organic frameworks[J] . We are testing a new system for linking publications to authors. As illustrated in Figure 1, the MOF Co-TPHS was synthesized by the coordination reaction of 2,3,6,7,10,11-triphenylenehexa(selenolate) ((TPHS) 6−) and cobaltous ions in the presence of base.Under inert atmosphere, the as-prepared (BBr) 3 TPHS was treated with ethyl alcohol and potassium hydroxide and stirred for a while. Is this your profile? In this work, we presented a new family of MOFs that combine significant porosity with electrical conductivity in a cubic framework. . Mohamad Hmadeh (2040910) Zheng Lu (123354) + 16 moreZheng Liu (28397) Felipe Gándara (1314675) Hiroyasu Furukawa (1288971) . You can help! The high quality nano-film of 2,3,6,7,10,11 . Conductive metal-organic frameworks (MOFs), with dispersed planar metal nodes and unique two-dimensional π-conjugated structures (13-15), have been intensively reported as potential promising electrocatalysts toward hydrogen evolution (16-18), oxygen evolution and reduction (19, 20), electric energy storage (21, 22), and so on.Despite fast charge transfer behaviors, conductive MOF in bulk . Mater. Porous Metal-Organic Framework Cu3 . 24, 3511-3513 (2012 . "Intrinsic Limitations of Atomic Layer Deposition for Pseudocapacitive Metal Oxides in Porous . Electrically conductive Metal-Organic Frameworks (MOFs) are promising materials for electronic devices, owing to their unique capability to adsorb guest molecules. . New porous crystals of extended metal-catecholates. C18H12O6. 1. The thin film not only can be precisely prepared in nanometer scale (20-70 nm), but also shows the pin-hole-free smooth surface. Chem. 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